LAUSR

Engineering Janus structures that possess anisotropic features in functions have attracted growing attention for a wide range of applications in sensors, catalysis, and biomedicine, and are yet usually designed at the nanoscale with distinct physical or chemical functionalities in their opposite sides. Inspired by the seamless integration of soft and hard materials in biological structures, here a mechanical Janus structure composed of soft and hard materials with a dramatic difference in mechanical properties at an additively manufacturable macroscale is presented. In the combination of extensive experimental, theoretical, and computational studies, the design principle of soft–hard materials integrated mechanical Janus structures is established and their unique rotation mechanism is addressed. The systematic studies of assembling the Janus structure units into superstructures with well‐ordered organizations by programming the local rotations are further shown, providing a direct route of designing superstructures by leveraging mechanical Janus structures with unique soft–hard material integration. Applications are conducted to demonstrate the features and functionalities of assembled superstructures with local ordered organizations in regulating and filtering acoustic wave propagations, thereby providing exemplification applications of mechanical Janus design in functional structures and devices.