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Oxide Semiconductor Phototransistor with Organolead Trihalide Perovskite Light Absorber

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A hybrid phototransistor is developed with solution-processed organolead trihalide perovskite (MAPbI3) capping indium gallium zinc oxide (IGZO), which well fuses the properties of the two materials in sensitive photodetecting and… Click to show full abstract

A hybrid phototransistor is developed with solution-processed organolead trihalide perovskite (MAPbI3) capping indium gallium zinc oxide (IGZO), which well fuses the properties of the two materials in sensitive photodetecting and high-mobility charge transporting, respectively. The MAPbI3-capped IGZO phototransistor demonstrates excellent responsivities of over 25 mA W−1 for lights with photon energies above the bandgap of perovskite light absorber. Besides the high sensitivity to light in both ultraviolet and visible regions, hybrid phototransistor maintains a fair on/off ratio of over 106 in the dark, and a field effect mobility of 12.9 cm2 V−1 s−1. The perovskite light absorber also obviates the long-standing problem for metal oxide phototransistor, the persistent photoconductivity behavior. Furthermore, fast transient response has been achieved by showing rise-time and fall-time within tens of milliseconds. The newly developed device opens variable optic-electric sensing applications for the integrated oxide–perovskite hybrid phototransistors.

Keywords: perovskite light; organolead trihalide; trihalide perovskite; oxide semiconductor; light absorber; phototransistor

Journal Title: Advanced electronic materials
Year Published: 2017

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