With a wide range of potential applications, the generation of nonclassical multiphoton and number states has attracted renewed interest recently. Here, a correlated quadphoton with seventh‐order nonlinear susceptibility is reported… Click to show full abstract
With a wide range of potential applications, the generation of nonclassical multiphoton and number states has attracted renewed interest recently. Here, a correlated quadphoton with seventh‐order nonlinear susceptibility is reported in which all four photons are simultaneously created via an eight‐wave mixing (EWM) process in an atomic medium. The efficiency of the pure EWM process is low, which results from the small order of magnitude of the seventh‐order nonlinear susceptibility (the quadphoton correlation with four periods corresponding to 8 channels and 12 resonance positions). But the EWM process has a strong dressing effect. It not only increases the nonlinear susceptibility, but also produces 15 or 16 resonance positions in the dressing state picture. In addition, with the energy conservation of these positions, 12 coherent channels can be generated in this system. According to the interference between multichannels of the quadphoton, the quadphoton coincidence count appears as a damped Rabi oscillation, which has eight or ten oscillation periods. If only the nonlinear optical response is considered, the coincidence counts of the quadphoton behave as a damped Rabi oscillation with periods that can be controlled by the dressing field. These outcomes may contribute to a new promising method for quantum communication.
               
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