Pulsed laser ablation of metal targets immersed in superfluid $$^4\hbox {He}$$4He is visualized by time-resolved shadowgraph photography and the products are analyzed by post-experiment atomic force microscopy (AFM) measurements. The… Click to show full abstract
Pulsed laser ablation of metal targets immersed in superfluid $$^4\hbox {He}$$4He is visualized by time-resolved shadowgraph photography and the products are analyzed by post-experiment atomic force microscopy (AFM) measurements. The expansion dynamics of the gaseous ablation half-bubble on the target surface appears underdamped and follows the predicted behavior for the thermally induced bubble growth mechanism. An inherent instability of the ablation bubble appears near its maximum radius and no tightly focused cavity collapse or rebound events are observed. During the ablation bubble retreat phase, the presence of sharp edges in the target introduces flow patterns that lead to the creation of large classical vortex rings. Furthermore, on the nanometer scale, AFM data reveal that the metal nanoparticles created by laser ablation are trapped in spherical vortex tangles and quantized vortex rings present in the non-equilibrium liquid.
               
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