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Age determination for uranium standard samples by 231Pa/235U radiochronometer

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Developing different model age determination methods of uranium sample could get more information on insight into source and suspected use in nuclear forensic investigation. A procedure for the determination of… Click to show full abstract

Developing different model age determination methods of uranium sample could get more information on insight into source and suspected use in nuclear forensic investigation. A procedure for the determination of model age of uranium sample using 231Pa/235U radiochronometer was reported. The 233Pa spike used in the procedure of 231Pa–235U model age determination was separated from in-house 237Np stock solution by using two TRU resin columns and three silica gel columns and calibrated by CRM U100. Model ages of CRM U010 and IRMM-1000b were presented. The model age of IRMM-1000b using 231Pa/235U radiochronometer were older than the literature reported results by 230Th/234U radiochronometer by amounts exceeded the expanded uncertainty.

Keywords: age determination; age; 231pa 235u; 235u radiochronometer

Journal Title: Journal of Radioanalytical and Nuclear Chemistry
Year Published: 2019

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