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Possible charge-density-wave signatures in the anomalous resistivity of Li-intercalated multilayer MoS2

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Abstract We fabricate ion-gated field-effect transistors (iFET) on mechanically exfoliated multilayer MoS2. We encapsulate the flake by Al2O3, leaving the device channel exposed at the edges only. A stable Li+… Click to show full abstract

Abstract We fabricate ion-gated field-effect transistors (iFET) on mechanically exfoliated multilayer MoS2. We encapsulate the flake by Al2O3, leaving the device channel exposed at the edges only. A stable Li+ intercalation in the MoS2 lattice is induced by gating the samples with a Li-based polymeric electrolyte above ∼ 330  K and the doping state is fixed by quenching the device to ∼ 300  K. This intercalation process induces the emergence of anomalies in the temperature dependence of the sheet resistance and its first derivative, which are typically associated with structural/electronic/magnetic phase transitions. We suggest that these anomalies in the resistivity of MoS2 can be naturally interpreted as the signature of a transition to a charge-density-wave phase induced by lithiation, in accordance with recent theoretical calculations.

Keywords: resistivity; density wave; charge density; mos2; multilayer mos2

Journal Title: Applied Surface Science
Year Published: 2018

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