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Abstract Bismuth oxybromide/molybdenum disulfide/graphene oxide (BiOBr/MoS2/GO) heterojunction composites were fabricated to modulate the adsorption ability and photocatalytic degradation performance toward oxytetracycline (OTC). The flowerlike BiOBr/MoS2/GO composites demonstrated excellent photocatalytic activies… Click to show full abstract
Abstract Bismuth oxybromide/molybdenum disulfide/graphene oxide (BiOBr/MoS2/GO) heterojunction composites were fabricated to modulate the adsorption ability and photocatalytic degradation performance toward oxytetracycline (OTC). The flowerlike BiOBr/MoS2/GO composites demonstrated excellent photocatalytic activies for the OTC degradation. Specifically, OTC, tetracycline, chlorotetracycline, and doxycycline were simultaneously removed with degradation rates higher than 98% under visible light irradiation within 40 min. Radical trapping experiments indicated that photogenerated holes (h+), hydroxyl radicals ( OH), and superoxide radicals ( O2−) played crucial roles in photocatalytic OTC degradation. Further, Possible transformation pathway and photocatalytic mechanism were proposed by investigating the intermediates in OTC degradation process.
Journal Title: Applied Surface Science
Year Published: 2021
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