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Enhanced energy-storage performance and temperature-stable dielectric properties of (1-x)[(Na0.5Bi0.5)0.95Ba0.05]0.98La0.02TiO3-xK0.5Na0.5NbO3 lead-free ceramics

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Abstract Polycrystalline (1-x)[(Na0.5Bi0.5)0.95Ba0.05]0.98La0.02TiO3-xK0.5Na0.5NbO3 systems were prepared using the solid-state reaction technique. Modification of (Na0.5Bi0.5)0.95Ba0.05]0.98La0.02TiO3 ceramic with a proper amount of K0.5Na0.5NbO3 can effectively improve the temperature-stable of dielectric properties. A… Click to show full abstract

Abstract Polycrystalline (1-x)[(Na0.5Bi0.5)0.95Ba0.05]0.98La0.02TiO3-xK0.5Na0.5NbO3 systems were prepared using the solid-state reaction technique. Modification of (Na0.5Bi0.5)0.95Ba0.05]0.98La0.02TiO3 ceramic with a proper amount of K0.5Na0.5NbO3 can effectively improve the temperature-stable of dielectric properties. A variation in dielectric constant is maintained smaller than ±5% from 80 to 300 °C accompanied with a low dielectric loss (≤0.04). The relaxor properties of the doped samples are significantly enhanced. A high energy storage density of 1.1 J/cm3 and efficiency ~80% at 90 kV/cm are achieved in the x = 0.05 composition. Hence, the as-prepared ceramics might be practical in dielectric constant which can work stably at a high temperature range and pulsed capacitors.

Keywords: 5bi0 95ba0; na0 5bi0; temperature; 98la0 02tio3; 95ba0 98la0; 5na0 5nbo3

Journal Title: Ceramics International
Year Published: 2019

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