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Bio-inspired incorporation of functionalized graphene oxide into carbon nanotube fibers for their efficient mechanical reinforcement

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Abstract An efficient strategy for the enhancement of mechanical properties of carbon nanotube (CNT) fibers is developed using functionalized graphene oxide with a quaternary ammonium (QA) group (QA-FGO). QA-FGO is… Click to show full abstract

Abstract An efficient strategy for the enhancement of mechanical properties of carbon nanotube (CNT) fibers is developed using functionalized graphene oxide with a quaternary ammonium (QA) group (QA-FGO). QA-FGO is designed to induce the π-cation interaction, one of the strongest interactions in living systems, with CNT fibers. Based on the strategy, the tensile strength (58 MPa), specific strength (0.49 N/tex), modulus (2.5 GPa) and toughness (1.1 MJ/m3) of CNT fibers are enhanced to 409 MPa, 0.65 N/tex, 13.4 GPa, and 10.1 MJ/m3, respectively. The reinforcement mechanism is systematically demonstrated with experimental and theoretical approaches.

Keywords: bio inspired; cnt fibers; functionalized graphene; graphene oxide; carbon nanotube; inspired incorporation

Journal Title: Composites Science and Technology
Year Published: 2019

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