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Dehydrogenation involved Coulomb explosion of molecular C 2 H 4 FBr in an intense laser field

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Abstract The dissociative double ionization (DDI) of molecular 1-fluo-2-bromoethane (FBE) in an intense laser field has been investigated by dc-slice imaging technology. The DDI channels involved with dehydrogenation are revealed… Click to show full abstract

Abstract The dissociative double ionization (DDI) of molecular 1-fluo-2-bromoethane (FBE) in an intense laser field has been investigated by dc-slice imaging technology. The DDI channels involved with dehydrogenation are revealed and it’s believed both the charge distribution and the bound character of real potential energy surfaces of parent ions play important roles in the dissociation process. The relationship between the potential energy surfaces of the precursor species and the photofragment ejection angles are also discussed and analyzed. Furthermore, the competition between the DDI channels has been studied and the C C bond cleavages dominate the DDI process at relative higher laser intensity.

Keywords: laser; laser field; dehydrogenation involved; involved coulomb; intense laser

Journal Title: Chemical Physics Letters
Year Published: 2018

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