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Dung beetle forewing-derived nitrogen and oxygen self-doped porous carbon for high performance solid-state supercapacitors

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Abstract Commercial supercapacitors are primarily assembled using carbon materials and biomass-derived carbon is one of the most promising carbon materials in the field of supercapacitors. To meet the growing market… Click to show full abstract

Abstract Commercial supercapacitors are primarily assembled using carbon materials and biomass-derived carbon is one of the most promising carbon materials in the field of supercapacitors. To meet the growing market demand for energy storage devices, a dung beetle forewing-derived carbon (DBFC) material is first prepared using simple a pyrolysis method. The as-prepared DBFC possesses a hierarchical porous structure, nitrogen and oxygen self-doping, and a large surface area. To investigate its electrochemical performance, the DBFC was used to prepare a supercapacitor electrode. A DBFC electrode prepared with a KOH to biomass-derived carbon mass ratio of 3:1 at 700 °C (DBFC-3-700) exhibits a high specific capacitance of 348 F g−1 at 0.5 A g−1 in 6 M KOH liquid electrolyte. The DBFC-3-700 electrode was further assembled into a solid-state symmetric supercapacitor that displays a high specific capacitance of 260 F g−1 at 0.5 A g−1, good cycle stability, and excellent rate capability. Furthermore, three solid-state supercapacitors connected in series can successfully power red light-emitting diodes, demonstrating potential applications in the field of portable and wearable devices.

Keywords: solid state; beetle forewing; carbon; dbfc; dung beetle

Journal Title: Journal of Alloys and Compounds
Year Published: 2022

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