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Base-free CO2 hydrogenation to formic acid over Pd supported on defective carbon nitride modified by microwave and acid treatments

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Abstract Graphitic carbon nitride (g-C3N4) is synthesized via pyrolyzing urea by hybrid microwave annealing (HMA) to support Pd catalyst for direct CO2 hydrogenation to formic acid under a base-free condition.… Click to show full abstract

Abstract Graphitic carbon nitride (g-C3N4) is synthesized via pyrolyzing urea by hybrid microwave annealing (HMA) to support Pd catalyst for direct CO2 hydrogenation to formic acid under a base-free condition. The HMA produces fragmented C3N4 sheets with abundant defects along their edges, because of the high annealing temperature (>900 oC) in an extremely short time (

Keywords: formic acid; base free; hydrogenation formic; carbon nitride; co2 hydrogenation; acid

Journal Title: Journal of Catalysis
Year Published: 2021

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