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Seasonal evolution of 7,10Be and 22Na in the near surface atmosphere of Cáceres (Spain).

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Cosmogenic radionuclides provide information about air masses exchanges between stratosphere and troposphere. The 7Be concentration in aerosols usually shows a seasonal variability, depending also of the climatic conditions. There are,… Click to show full abstract

Cosmogenic radionuclides provide information about air masses exchanges between stratosphere and troposphere. The 7Be concentration in aerosols usually shows a seasonal variability, depending also of the climatic conditions. There are, however, fewer data available of the behavior of other cosmogenic radionuclides, such as 10Be and 22Na. In this work about 7 years of aerosols collected in Cáceres (Spain) were analyzed. The 7Be concentration was higher than 22Na and 10Be, being the 22Na/7Be and 10Be/7Be ratios (1.16 ± 0.02)·10-4 and (1.5 ± 0.3)·10-4 respectively. For the 22Na/7Be, a seasonal variation was observed, being higher in spring/summer. Seasonal variation of 7Be and 22Na were explained using a model taking into account local values of the solar radiation, rainfall and dry deposition. The effective residence time for 7Be and 22Na were (9.9 ± 1.0) and (11.3 ± 1.4) d respectively. Both 7Be and 22Na seemed to decrease with increasing number of sunspots, although it was not statistically significant probably due to the low solar activity reported in the analyzed period.

Keywords: 10be 22na; seasonal evolution; evolution 10be; 22na near; ceres spain; 7be 22na

Journal Title: Journal of environmental radioactivity
Year Published: 2019

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