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Enhanced single-mode lasers of all-inorganic perovskite nanocube by localized surface plasmonic effect from Au nanoparticles

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Abstract Miniaturized laser sources recently attracted considerable interests as their potential applications in optical communication, data storage, and imaging. However, high cavity losses induced by size reduction from the gain… Click to show full abstract

Abstract Miniaturized laser sources recently attracted considerable interests as their potential applications in optical communication, data storage, and imaging. However, high cavity losses induced by size reduction from the gain medium would lead high lasing threshold. In this work, the enhanced optical properties of CsPbBr3 perovskite nanocubes by using localized surface plasmonic effect of Au nanoparticles (NPs) were investigated. The integration of Au NPs in the poly (3, 4-ethylenedioxy-thiophene): poly (styrenesulfonate) PEDOT: PSS layer induces obviously enhancement both in the absorption and photoluminescence (PL) of CsPbBr3 perovskite nanocubes. Importantly, the lasing threshold of CsPbBr3 perovskite nanocubes is significantly reduced by ~ 33%. This study suggests that the lead halide perovskites hybridized with plasmonic nanomaterials would be promising candidates for laser devices and other optoelectronic devices with high efficiency.

Keywords: effect nanoparticles; surface plasmonic; localized surface; plasmonic effect

Journal Title: Journal of Luminescence
Year Published: 2019

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