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Magnetization process and magnetocaloric effect in geometrically frustrated Ising antiferromagnet and spin ice models on a ‘Star of David’ nanocluster

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Abstract Magnetic and magnetocaloric properties of geometrically frustrated antiferromagnetic Ising (IA) and ferromagnetic spin ice (SI) models on a nanocluster with a ‘Star of David’ topology, including next-nearest-neighbor (NNN) interactions,… Click to show full abstract

Abstract Magnetic and magnetocaloric properties of geometrically frustrated antiferromagnetic Ising (IA) and ferromagnetic spin ice (SI) models on a nanocluster with a ‘Star of David’ topology, including next-nearest-neighbor (NNN) interactions, are studied by an exact enumeration. In an external field applied in characteristic directions of the respective models, depending on the NNN interaction sign and magnitude, the ground state magnetization of the IA model is found to display up to three intermediate plateaus at fractional values of the saturation magnetization, while the SI model shows only one zero-magnetization plateau and only for the antiferromagnetic NNN coupling. A giant magnetocaloric effect is revealed in the IA model with the NNN interaction either absent or equal to the nearest-neighbor coupling. The latter is characterized by abrupt isothermal entropy changes at low temperatures and infinitely fast adiabatic temperature variations for specific entropy values in the processes when the magnetic field either vanishes or tends to the critical values related to the magnetization jumps.

Keywords: ice models; geometrically frustrated; magnetocaloric effect; magnetization; star david; spin ice

Journal Title: Journal of Magnetism and Magnetic Materials
Year Published: 2017

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