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Uranium solubility and speciation in reductive soda-lime aluminosilicate glass melts

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Abstract Uranium solubility in aluminosilicate melts of the Na2O-CaO-Al2O3-SiO2 system with two different Na/Ca ratios was studied at temperatures of 1250–1400°C and under various redox conditions. A closed thermochemical reactor… Click to show full abstract

Abstract Uranium solubility in aluminosilicate melts of the Na2O-CaO-Al2O3-SiO2 system with two different Na/Ca ratios was studied at temperatures of 1250–1400°C and under various redox conditions. A closed thermochemical reactor was used to control the alkali metal activity (sodium oxide content) and the oxygen fugacity imposing the reducing environment on the glass melt (10−5 atm

Keywords: glass; uranium solubility; solubility speciation; aluminosilicate; solubility; speciation reductive

Journal Title: Journal of Nuclear Materials
Year Published: 2020

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