LAUSR

Long-term monitoring is essential for revealing pollution trends, but relevant studies in the Antarctic remain limited. In this study, a seven-year continuous monitoring of polycyclic aromatic hydrocarbons (PAHs) in the atmosphere and soil was carried out at the Fildes Peninsula, Antarctica. Average concentrations of Σ15PAHs were 7134.491 pg/m3 and 61.093 ng/g in air and soil, respectively. A declining trend was observed for Σ15PAHs in air during the 2013-2019 summer, but this was not found in soil. Potential sources of PAHs in the Fildes Peninsula were identified by PMF modeling, correlation analysis, air mass back-trajectories and component analysis. The results showed that PAHs in the gas phase were more easily influenced by long-range atmospheric transport (LRAT) than in the particle phase. Moreover, temperature played a key role in the PAHs concentration in particle phase. Occurrence of Σ15PAHs in soil was mainly attributed to local sources including fossil fuel combustion and spilling.