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Acoustic frequency and optimum sonochemical production at single and multi-bubble scales: A modeling answer to the scaling dilemma

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Highlights • Sonochemical production (SP) is modeled and simulated at bubble and reactor scales.• Monotonous variation of SP versus frequency is observed at single bubble scale.• Absolute optimum is observed… Click to show full abstract

Highlights • Sonochemical production (SP) is modeled and simulated at bubble and reactor scales.• Monotonous variation of SP versus frequency is observed at single bubble scale.• Absolute optimum is observed at 200 kHz at reactor scale for all products, except HO•.• HO• attains the maximum production within the sonochemical reactor at 300 kHz.• Predominant species, namely HO2•, HO• and O3, manifests a clear rebound at 500 kHz.• The scalability of SP is discussed based on the mass focusing factor.

Keywords: sonochemical production; production; optimum sonochemical; frequency optimum; acoustic frequency

Journal Title: Ultrasonics Sonochemistry
Year Published: 2020

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