Efficient thermally activated delayed fluorescence materials based on the multiple resonance effect were synthesized by nucleophilic substitution and electrophilic C-H borylation, featuring a small energy gap between the singlet and… Click to show full abstract
Efficient thermally activated delayed fluorescence materials based on the multiple resonance effect were synthesized by nucleophilic substitution and electrophilic C-H borylation, featuring a small energy gap between the singlet and triplet state, high photoluminescence quantum yield, and narrow emission band. Organic light-emitting diodes employing these materials as emitters exhibited sky-blue emission with a high external quantum efficiency of 21.4% and a narrow full width at half-maximum of 33 nm.
               
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