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Improving Quantum Well Tube Homogeneity Using Strained Nanowire Heterostructures

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Bottom-up grown nanostructures often suffer from significant dimensional inhomogeneity, and for quantum confined heterostructures, this can lead to a corresponding large variation in electronic properties. A high-throughput characterization methodology is… Click to show full abstract

Bottom-up grown nanostructures often suffer from significant dimensional inhomogeneity, and for quantum confined heterostructures, this can lead to a corresponding large variation in electronic properties. A high-throughput characterization methodology is applied to >15,000 nanoskived sections of highly strained GaAsP/GaAs radial core/shell quantum well heterostructures revealing high emission uniformity. While scanning electron microscopy shows a wide nanowire diameter spread of 540–60+60 nm, photoluminescence reveals a tightly bounded band-to-band transition energy of 1546–3+4 meV. A highly strained core/shell nanowire design is shown to reduce the dependence of emission on the quantum well width variation significantly more than in the unstrained case.

Keywords: tube homogeneity; homogeneity using; improving quantum; using strained; well tube; quantum well

Journal Title: ACS Applied Materials & Interfaces
Year Published: 2023

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