LAUSR

We demonstrate graphene-functionalized self-phase-locking of laser pulses for a dramatically elevated repetition rate by employing an intrinsic resonating structure in a fiber ring laser cavity, the modes thereby satisfying the phase-matching condition passively, through both the resonator and the laser cavity. Graphene is directly synthesized around a 1-mm-diameter Cu wire catalyst, avoiding the deleterious transfer process. The wire provides a form factor to the fiber ring resonator as a versatile winding hub, guaranteeing damage-minimized and recyclable contact of the synthesized graphene with a diameter-controlled optical microfiber. In-depth analysis of the graphene confirms the optical nonlinearity critically required for pulse formation. The laser-graphene interaction, the intermode phase-locking function of graphene, and the pulse formation with the resonator are systematically elucidated to explain the experimentally generated laser pulses at a repetition rate of 57.8 gigahertz (GHz). Additionally, tunability of the repetition rate up to 1.5 GHz by the photothermal effect of graphene is demonstrated.