It is highly desirable to fabricate two-dimensional ferromagnetic membranes based on orthodox magnetic elements because of their inherent magnetic properties. In this work, we report on two superstructures including a… Click to show full abstract
It is highly desirable to fabricate two-dimensional ferromagnetic membranes based on orthodox magnetic elements because of their inherent magnetic properties. In this work, we report on two superstructures including a honeycomb-like lattice and identical nanocluster arrays formed by depositing Fe on Sb(111). Combined with first-principles calculations, both detailed atomic structures have been clarified. The honeycomb structure consists of a single layered Fe-Sb phase, and the cluster phase is assigned as a (3 × 3) Fe3Sb7 superlattice. Both structural phases exhibit high magnetic moments localized on d bands of Fe. Our results provide a method to fabricate 2D magnetic superstructures possessing great potential in the realization of the Haldane model, spintronics applications, and single atom catalysis.
               
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