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Cu-Doped MoSe2 Monolayer: A Novel Candidate for Dissolved Gas Analysis in Transformer Oil

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Dissolved gas analysis (DGA) in transformer oil is a workable approach to evaluate the operation status of transformers. In this paper, we proposed a Cu-doped Se-vacancy MoSe2 (Cu-MoSe2) monolayer as… Click to show full abstract

Dissolved gas analysis (DGA) in transformer oil is a workable approach to evaluate the operation status of transformers. In this paper, we proposed a Cu-doped Se-vacancy MoSe2 (Cu-MoSe2) monolayer as a promising sensing material for DGA based on first-principles theory. Three typical dissolved gases, namely, CO, C2H2, and C2H4, are the representatives to investigate the potential of the Cu-MoSe2 monolayer upon their adsorption and sensing. Our results indicate that Cu-doping causes strong n-doping for the Se-vacancy MoSe2 monolayer, and the Cu-MoSe2 monolayer exhibits strong chemisorption the three gas molecules, with a calculated adsorption energy (Ead) of −1.25, −1.06, and −1.16 eV, respectively. Such strong interactions lead to remarkable changes in the electrical conductivity of the Cu-MoSe2 monolayer, allowing its application as a resistance-type sensor. Besides, work function (WF) analysis shows the potential of the Cu-MoSe2 monolayer as a promising field-effect transistor sensor as well. It is our hope that our work can stimulate more leading-edge studies of the TM-doped MoSe2 monolayer for sensing applications in many fields.

Keywords: dissolved gas; analysis; mose2 monolayer; monolayer

Journal Title: ACS Omega
Year Published: 2020

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