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Designing Multifunctional Coatings for Cost-Effectively Sustainable Water Remediation

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Multifunctional coatings derived from bioinspired dopamine (DA) have attracted a lot of attention for water environmental remediation recently. Nevertheless, the high cost of DA monomers seriously hampers their broad application.… Click to show full abstract

Multifunctional coatings derived from bioinspired dopamine (DA) have attracted a lot of attention for water environmental remediation recently. Nevertheless, the high cost of DA monomers seriously hampers their broad application. Herein, an elegant multifunctional coating, which could be deployed as a selective adsorbent or loose nanofiltration membrane for removing of dyes and antibiotics from water, was designed based on the Michael-addition and Schiff-base reactions between cost-effective plant-derived gallic acid (GA) and branched polyethylenimine (PEI) at room temperature. Aside from the extremely low cost of GA (about 5% of that of DA), the resultant GA/PEI coatings possessed much better performance than DA/PEI coatings. When deployed as a dye adsorbent, the bioinspired GA/PEI coatings exhibited much higher selectivity, showing 40% increase in anionic dye adsorptive capability and 30% decline in cationic dye adsorptive capability compared with DA/PEI coatings. When applied as a nanofiltration membra...

Keywords: multifunctional coatings; pei coatings; designing multifunctional; water; remediation; cost

Journal Title: ACS Sustainable Chemistry & Engineering
Year Published: 2018

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