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Lotus-Leaf-Derived Activated-Carbon-Supported Nano-CdS as Energy-Efficient Photocatalysts under Visible Irradiation

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Lotus-leaf-derived activated carbon materials (denoted as LAC-T) were fabricated at different temperatures (T = 600, 700, and 800 °C), which resulted in carbonaceous materials with various microstructures and porosity. BET… Click to show full abstract

Lotus-leaf-derived activated carbon materials (denoted as LAC-T) were fabricated at different temperatures (T = 600, 700, and 800 °C), which resulted in carbonaceous materials with various microstructures and porosity. BET surface area of LAC-T increased from 1184 m2 g–1 to 1807 m2 g–1 with activation temperatures that varied from 600 °C to 800 °C. These microporous carbonaceous materials were subsequently advanced as ideal platforms for cadmium sulfide (CdS) composite photocatalysts, through the deposition of nano-CdS precursors on LAC-T supports (CdS@LAC-T). It was revealed that the CdS@LAC-T nanocomposites displayed enhanced photocatalytic efficiency, in comparison with the nano-CdS, toward the degradation of various organic dyes under visible light. More specifically, CdS@LAC-800, prepared from a carbonaceous support with the highest BET, gave the best photocatalytic efficiency. Estimated band gap energy for CdS@LAC-800 (2.01 eV) was considerably lower than that of nano-CdS (2.22 eV), which was among ...

Keywords: lotus leaf; nano cds; derived activated; leaf derived; cds lac; activated carbon

Journal Title: ACS Sustainable Chemistry & Engineering
Year Published: 2018

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