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Structure of spin excitations in heavily electron-doped Li0.8Fe0.2ODFeSe superconductors

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Heavily electron-doped iron-selenide high-transition-temperature (high-Tc) superconductors, which have no hole Fermi pockets, but have a notably high Tc, have challenged the prevailing s± pairing scenario originally proposed for iron pnictides… Click to show full abstract

Heavily electron-doped iron-selenide high-transition-temperature (high-Tc) superconductors, which have no hole Fermi pockets, but have a notably high Tc, have challenged the prevailing s± pairing scenario originally proposed for iron pnictides containing both electron and hole pockets. The microscopic mechanism underlying the enhanced superconductivity in heavily electron-doped iron-selenide remains unclear. Here, we used neutron scattering to study the spin excitations of the heavily electron-doped iron-selenide material Li0.8Fe0.2ODFeSe (Tc = 41 K). Our data revealed nearly ring-shaped magnetic resonant excitations surrounding (π, π) at ∼21 meV. As the energy increased, the spin excitations assumed a diamond shape, and they dispersed outward until the energy reached ∼60 meV and then inward at higher energies. The observed energy-dependent momentum structure and twisted dispersion of spin excitations near (π, π) are analogous to those of hole-doped cuprates in several aspects, thus implying that such spin excitations are essential for the remarkably high Tc in these materials.The microscopic mechanism underlying an enhanced superconductivity in electron-doped iron selenide superconductor remains unclear. Here, Pan et al. report the spin excitations of Li0.8Fe0.2ODFeSe, revealing analogous momentum structure and dispersion to hole-doped cuprates.

Keywords: iron; heavily electron; spin excitations; electron doped; li0 8fe0; 8fe0 2odfese

Journal Title: Nature Communications
Year Published: 2017

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