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At high loading, methanol reacts under ambient conditions with acidic hydroxyls of H-ZSM-5 to methoxylate framework oxygen; while a significant proportion remains hydrogen bonded to the framework with a protonated… Click to show full abstract
At high loading, methanol reacts under ambient conditions with acidic hydroxyls of H-ZSM-5 to methoxylate framework oxygen; while a significant proportion remains hydrogen bonded to the framework with a protonated geometry. The findings not only explain the data which have been published so far, but also pave a way forward for potential unravelling of the initial reaction steps in the relevant chemical processes.
Keywords:
zsm;
zeolite zsm;
room temperature;
zsm operando;
methoxylation zeolite;
temperature methoxylation
Journal Title: Chemical communications
Year Published: 2018
Link to full text (if available)
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Journal Title: Chemical communications
Year Published: 2018
Link to full text (if available)
Share on Social Media: Sign Up to like & get
recommendations!