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Nanosized hierarchical TS-1 zeolites with intercrystalline and intracrystalline meso-/macropores have been successfully synthesised by amino acid-assisted strategy under two-step rota-crystallization conditions. Compared to micron-sized microporous TS-1 zeolites, amino acid-directed hierarchical… Click to show full abstract
Nanosized hierarchical TS-1 zeolites with intercrystalline and intracrystalline meso-/macropores have been successfully synthesised by amino acid-assisted strategy under two-step rota-crystallization conditions. Compared to micron-sized microporous TS-1 zeolites, amino acid-directed hierarchical materials exhibit remarkably enhanced catalytic activity in oxidative desulfurization reactions owing to the improved accessibility of reactants to the microporous space of zeolites.
Journal Title: Inorganic chemistry frontiers
Year Published: 2020
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