The discovery of facile methods to create complex lamellar structures in hydrogels, which mimic the exquisite structures in nature, remains a great challenge. In this work, an ordered lamellar structured… Click to show full abstract
The discovery of facile methods to create complex lamellar structures in hydrogels, which mimic the exquisite structures in nature, remains a great challenge. In this work, an ordered lamellar structured hydrogel from the stimuli-responsive amino-polysaccharide chitosan is fabricated by an electro-assembly process, during which the diffusion of OH- and the electrophoresis of the chitosan chains play important roles. Importantly, a complex ordered/disordered structure of chitosan hydrogel can be regulated with high fidelity by programming the input electrical signals.
               
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