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In this study, we construct a Cu@ZrO2 heterogenous structure as a new catalyst that achieves a large NH3 yield of 15.4 mg h-1 mg-1cat. and a high faradaic efficiency of… Click to show full abstract
In this study, we construct a Cu@ZrO2 heterogenous structure as a new catalyst that achieves a large NH3 yield of 15.4 mg h-1 mg-1cat. and a high faradaic efficiency of 67.6% at -0.7 V vs. RHE in 0.1 M PBS with 0.1 M NaNO3, and it also shows excellent electrochemical durability and structural stability. Theoretical calculations reveal an extremely low adsorption energy of -1.54 eV at Cu surfaces and Cu can significantly reduce the applied overpotential and correspondingly promote the catalytic activity.
Keywords:
efficient electrocatalytic;
nanofibers enable;
enable efficient;
heterogenous zro2;
zro2 nanofibers;
zro2
Journal Title: Chemical communications
Year Published: 2022
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Journal Title: Chemical communications
Year Published: 2022
Link to full text (if available)
Share on Social Media: Sign Up to like & get
recommendations!