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Hybrid nanoarrays of Cu-MOFs@H-substituted graphdiyne with various levels of Lewis acidity for nitrate electroreduction.

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To mimic enzymes in nature, a set of hybrid nanoarrays of Cu-MOFs sealed in hydrogen-substituted graphdiyne has been developed in order to serve as Lewis-acid-promoted catalysts. By regulating the electron-withdrawing… Click to show full abstract

To mimic enzymes in nature, a set of hybrid nanoarrays of Cu-MOFs sealed in hydrogen-substituted graphdiyne has been developed in order to serve as Lewis-acid-promoted catalysts. By regulating the electron-withdrawing capability of the ligands bridging Cu2+ sites, these Cu-MOFs provided different levels of Lewis acidity toward nitrate affinity, a feature crucial for nitrate-to-ammonia conversion.

Keywords: hybrid nanoarrays; substituted graphdiyne; levels lewis; nanoarrays mofs; lewis acidity

Journal Title: Chemical communications
Year Published: 2023

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