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Mode-dependent energy exchange between near- and far-field through silicon-supported single silver nanorods.

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Optical antenna effects endow plasmonic nanoparticles with the capability to enhance and control various types of light-matter interaction. Most reported plasmonic systems can be regarded as single-channel nanoantennas, which rely… Click to show full abstract

Optical antenna effects endow plasmonic nanoparticles with the capability to enhance and control various types of light-matter interaction. Most reported plasmonic systems can be regarded as single-channel nanoantennas, which rely only on a bright dipole plasmon mode for energy exchange between near- and far-field. Herein we demonstrate a dual-channel plasmonic system that can separate the excitation and emission processes into two energy exchange pathways mediated by the different plasmon modes, offering a higher degree of freedom for the manipulation of light-matter interaction. Our system, consisting of high-aspect-ratio Ag nanorods and Si substrates, can support a series of bright and dark plasmon modes with distinct near- and far-field properties and generate relatively intensive local field enhancement in the gap region. As a proof-of-principle, we take plasmon-enhanced fluorescence of dye molecules as an example to reveal the energy exchange mechanism in the dual-channel plasmonic system. Such a system is potentially also useful for manipulating other types of light-matter interaction. Our work represents a step toward the utilization of a broader class of plasmon resonance for the development of optical antennas and various on-chip nanophotonic components.

Keywords: near far; far field; energy; energy exchange

Journal Title: Nanoscale
Year Published: 2022

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