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Assembly of Fluorinated Benzodiazepines via Rh(III)-Catalysed [5+2] Annulation of N-Benzo[d]imidazole Indolines with 2,2-Difluorovinyl Tosylate

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Herein, we have realized an efficient and solvent-tunable Rh(III)-catalyzed [5+2] annulation of N-benzo[d]imidazole indolines with 2,2-difluorovinyl tosylate that presented an unusual 1,2-regioselectivity for the chemodivergent construction of monofluorinated and gem-difluorinated... Click to show full abstract

Herein, we have realized an efficient and solvent-tunable Rh(III)-catalyzed [5+2] annulation of N-benzo[d]imidazole indolines with 2,2-difluorovinyl tosylate that presented an unusual 1,2-regioselectivity for the chemodivergent construction of monofluorinated and gem-difluorinated...

Keywords: imidazole indolines; indolines difluorovinyl; annulation benzo; benzo imidazole; iii; difluorovinyl tosylate

Journal Title: New Journal of Chemistry
Year Published: 2023

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