Eutectogels are stretchable ionic conductors extensively developed in recent years, owing to their distinct advantages of low cost, non-volatility, non-toxicity, and outstanding biocompatibility. However, the susceptibility to humidity caused by… Click to show full abstract
Eutectogels are stretchable ionic conductors extensively developed in recent years, owing to their distinct advantages of low cost, non-volatility, non-toxicity, and outstanding biocompatibility. However, the susceptibility to humidity caused by the exchange of water molecules between the interiors of eutectogels and the external environment greatly restricts their practical applications. Here, a dip-coating strategy is proposed to fabricate a P(MEA-co-IBA) elastomer-coated P(AAC-co-AAM) eutectogel to achieve satisfactory humidity-resistant capability. The hydrophobic elastomer coating significantly suppresses water exchange without harming the stretchability (>500%) and conductivity of the eutectogel. Strong adhesion forms at the eutectogel-coating interface due to the formation of an interpenetrating layer. The superior electromechanical performances of encapsulated eutectogels enable stretchable ionotronic devices with stable electrical performance (>1 h) and remarkable water-droplet/moist resistances during static/dynamic loadings. A humidity-resistant encapsulated eutectogel-based wearable strain sensor is further demonstrated. The proposed humidity-resistant eutectogels are promising candidates for soft and wearable ionotronics for practical applications.
               
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