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Anisotropic ultrafast optical response of terahertz pumped graphene

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We have measured the ultrafast anisotropic optical response of highly doped graphene to an intense single cycle terahertz pulse. The temporal shape of the signal is similar to that of… Click to show full abstract

We have measured the ultrafast anisotropic optical response of highly doped graphene to an intense single cycle terahertz pulse. The temporal shape of the signal is similar to that of the pump terahertz electric field modulus. It grows with increasing carrier density and demonstrates a specific nonlinear dependence on the electric field strength. To describe the signal, we have developed a theoretical model that is based on the energy and momentum balance equations and takes into account optical phonons of graphene and substrate. According to the theory, the anisotropic response is caused by the displacement of the electronic momentum distribution from zero momentum induced by the pump electric field in combination with polarization dependence of the matrix elements of interband optical transitions.

Keywords: response; anisotropic ultrafast; ultrafast optical; terahertz; optical response; electric field

Journal Title: Applied Physics Letters
Year Published: 2019

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