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Femtosecond imbalanced time-stretch spectroscopy for ultrafast gas detection

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Dual-comb spectroscopy is a promising method for precise optical spectrum analysis with fast data acquisition speed. Here, avoiding using a dual-comb source, femtosecond imbalanced time-stretch spectroscopy with a simple optical… Click to show full abstract

Dual-comb spectroscopy is a promising method for precise optical spectrum analysis with fast data acquisition speed. Here, avoiding using a dual-comb source, femtosecond imbalanced time-stretch spectroscopy with a simple optical layout is proposed and demonstrated. Time-stretch interferometry from one femtosecond laser builds mapping from the optical frequency domain to the radio frequency regime. In experiment, the absorption line of a hydrogen cyanide cell is encoded in the probing arm of a Mach–Zehnder interferometer (MZI). The down-converted radio frequency comb is transformed from a periodically chirped waveform, which is the interferogram of the MZI with different dispersion values on two arms. In a single measurement, the optical frequency comb with a span of 112.5 GHz is down-converted to a range of about 20.8 GHz in the radio frequency domain with a comb spacing equal to the laser repetition frequency of 100 MHz. By turning the optical filter, a spectrum range around 2 THz is analyzed. The acquired optical spectrum resolution is 540 MHz.

Keywords: frequency; comb; spectroscopy; time stretch

Journal Title: Applied Physics Letters
Year Published: 2019

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