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Stabilization and manipulation of in-plane polarization in a ferroelectric|dielectric superlattice

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We investigate in-plane ferroelectricity in an epitaxial ferroelectric |dielectric PbTiO 3 | SrTiO 3 (PTO |STO) superlattice under tensile strain. Using a combination of x-ray diffraction and piezoresponse force microscopy,… Click to show full abstract

We investigate in-plane ferroelectricity in an epitaxial ferroelectric |dielectric PbTiO 3 | SrTiO 3 (PTO |STO) superlattice under tensile strain. Using a combination of x-ray diffraction and piezoresponse force microscopy, we identify a strain-induced periodic in-plane nanoscale domain architecture with polarization along the base diagonals of the PTO unit cell. We scrutinize its switching behavior using local in-plane trailing fields from the scanning-probe tip. For an electric field pointing in the polarization direction of a specific domain state, we create stable single-domain areas of in-plane polarization at the scale of tens of micrometers. Our findings on controlling robust in-plane ferroelectricity in ultrathin ferroelectric layers can help one to develop device concepts unaffected by the detrimental effects of the depolarizing field.

Keywords: stabilization manipulation; superlattice; polarization; ferroelectric dielectric; plane; plane polarization

Journal Title: Journal of Applied Physics
Year Published: 2021

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