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Efficient generation of UV-enhanced intense supercontinuum in solids: Toward sub-cycle transient

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Ultrabroadband generation of white-light continuum spanning from ultraviolet to near-infrared (375–920 nm) is demonstrated by using induced-phase modulation between two-color femtosecond pulses in multiple thin plates. The fundamental wave and its… Click to show full abstract

Ultrabroadband generation of white-light continuum spanning from ultraviolet to near-infrared (375–920 nm) is demonstrated by using induced-phase modulation between two-color femtosecond pulses in multiple thin plates. The fundamental wave and its second-harmonic wave from one Ti:sapphire chirped-pulse amplifier are injected into nine 100 μm-thick fused silica plates. When the two pulses are temporally and spatially optimized in the plates, an intense supercontinuum is efficiently achieved by utilizing self-phase modulation and self-steepening together with induced-phase modulation. As a result, using 1 kHz, 1 mJ, and 35 fs pulses at 800 nm as the pump, we demonstrate the generation of 0.6 mJ white-light pulses with an ultra-broad bandwidth supporting 1.6 fs transform-limited pulses corresponding to 0.6-optical-cycle at a central wavelength of 750 nm. Analysis of the calculated spectrum fits the experimental results well, and the pulse is quasi-linearly chirped and compressible. The resulting intense robust supercontinuum could be a promising light source for an ever greater degree of tailored optical waveform coherent control in new parameter spaces.

Keywords: efficient generation; generation; cycle; intense supercontinuum; phase modulation; supercontinuum

Journal Title: Applied Physics Letters
Year Published: 2021

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