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Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi2Sr2LaCuO6+δ

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Significance Charge-density waves (CDWs) are a ubiquitous form of electron density modulation in cuprate superconductors. Unveiling the nature of quasistatic CDWs and their dynamical excitations is crucial for understanding their… Click to show full abstract

Significance Charge-density waves (CDWs) are a ubiquitous form of electron density modulation in cuprate superconductors. Unveiling the nature of quasistatic CDWs and their dynamical excitations is crucial for understanding their origin––similar to the study of antiferromagnetism in cuprates. However, dynamical CDW excitations remain largely unexplored due to the limited availability of suitable experimental probes. Here, using resonant inelastic X-ray scattering, we observe dynamical CDW excitations in Bi2Sr2LaCuO6+δ (Bi2201) superconductors through its interference with the lattice. The distinct anomalies of the bond-buckling and the bond-stretching phonons allow us to draw a clear picture of funnel-shaped dynamical CDW excitations in Bi2201. Our results of the interplay between CDWs and the phonon anomalies shed light on the nature of CDWs in cuprates. Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate underdoped Bi2Sr1.4La0.6CuO6+δ using resonant inelastic X-ray scattering (RIXS) and find that a short-range CDW exists at both Cu and O sublattices in the copper-oxide (CuO2) planes with a comparable periodicity and correlation length. Furthermore, we uncover bond-stretching and bond-buckling phonon anomalies concomitant to the CDWs. Comparing to slightly overdoped Bi2Sr1.8La0.2CuO6+δ, where neither CDWs nor phonon anomalies appear, we highlight that a sharp intensity anomaly is induced in the proximity of the CDW wavevector (QCDW) for the bond-buckling phonon, in concert with the diffused intensity enhancement of the bond-stretching phonon at wavevectors much greater than QCDW. Our results provide a comprehensive picture of the quasistatic CDWs, their dispersive excitations, and associated electron-phonon anomalies, which are key for understanding the competing electronic instabilities in cuprates.

Keywords: bond; charge density; cdw; density; phonon anomalies; cdws

Journal Title: Proceedings of the National Academy of Sciences of the United States of America
Year Published: 2020

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