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Pressure Induced Insulator to Metal Transition in Quantum Spin Liquid Candidate NaYbS2

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Pressure induced insulator to metal transition followed by the appearance of superconductivity has been observed recently in inorganic quantum spin liquid candidate NaYbSe2. In this letter, we study the properties… Click to show full abstract

Pressure induced insulator to metal transition followed by the appearance of superconductivity has been observed recently in inorganic quantum spin liquid candidate NaYbSe2. In this letter, we study the properties of isostructural compound NaYbS2 under pressure. It is found that the resistance of NaYbS2 single crystal exhibits an insulating state below 82.9 GPa, but with a drop of more than six orders of magnitude at room temperature. Then a minimum of resistance is observed at about 100.1 GPa and it moves to lower temperature with further compression. Finally, a metallic state in the whole temperature range is observed at about 130.3 GPa accompanied a non-Fermi liquid behavior below 100 K. The insulator to metal transition, non-monotonic resistance feature and non-Fermi liquid behavior of NaYbS2 under pressure is similar to those of NaYbSe2, suggesting that these phenomena might be the universal properties in NaLnCh2 (Ln = rare earth, Ch = O, S, Se) system.

Keywords: pressure; insulator metal; metal transition

Journal Title: Chinese Physics B
Year Published: 2023

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