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A finite-time fluctuation theorem for the diffusion-influenced surface reaction is investigated for spherical and Janus catalytic particles. The finite-time rates and thermodynamic force are analytically calculated by solving diffusion equations… Click to show full abstract
A finite-time fluctuation theorem for the diffusion-influenced surface reaction is investigated for spherical and Janus catalytic particles. The finite-time rates and thermodynamic force are analytically calculated by solving diffusion equations with the special boundary conditions of the finite-time fluctuation theorem. Theory is compared with numerical simulations carried out with two different methods: a random walk algorithm and multiparticle collision dynamics.
Keywords:
finite time;
time fluctuation;
fluctuation theorem;
time
Journal Title: Journal of Statistical Mechanics: Theory and Experiment
Year Published: 2018
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Journal Title: Journal of Statistical Mechanics: Theory and Experiment
Year Published: 2018
Link to full text (if available)
Share on Social Media: Sign Up to like & get
recommendations!