LAUSR

Atmospheric NO x concentrations are declining steadily due to successful abatement strategies predominantly targeting combustion sources. On the European continent, total NO x emissions fell by 55% between 1990 and 2017, but only modest reductions were achieved from the agricultural sector; with 7.8% from 20 Eastern European countries and 19.1% from 22 Western European countries. Consequently, the share of agricultural NO x emissions for these 42 European countries have increased from 3.6% to 7.2%. These values are highly uncertain due to serious lack of studies from agricultural soils and manure management. The emission factor (EFNO 1.33%), currently used for calculating soil NO x emissions from European agricultural categories ‘N applied to soils’ and ‘manure management’ was evaluated here by including recently published data from temperate climate zones. The newly calculated EFNO (average 0.60%, 0.0625th%/0.5475th%, n = 65 studies) is not notably different from the current value, given the large uncertainties associated with the small pool of studies, and therefore continued use of EFNO (1.33%) is recommended until more data become available. An assessment of the contribution of agricultural and non-agricultural NO x sources found that of the 42 European countries, the 8 most populated countries achieved considerable reductions (1990–2017) from categories ‘non-agricultural sources’ (55%), ‘N applied to soils’ (43%) and ‘manure management’ (1.2%), compared to small reductions from the remaining 34 countries. Forests are also large sources of soil NO x . On average, emissions from Eastern European forests were 4 times larger than from ‘N applied agricultural soil’, whereas Western European NO x emissions from ‘N applied agricultural soil’ were two times larger than from forest soils. Given that non-agricultural sources of NO x continue to decline, soil related emissions from agriculture, forests and manure management become more important, and require rigorous investigation in order to improve atmospheric pollution forecasts.