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Competition between dynamic resonance and internal conversion in strong-field molecular ionization with chirped ultrafast laser pulses

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The authors show theoretically and experimentally how the time-varying phase or frequency of a chirped strong-field ultrafast laser pulse can be used to control the ionization yield to different ionic… Click to show full abstract

The authors show theoretically and experimentally how the time-varying phase or frequency of a chirped strong-field ultrafast laser pulse can be used to control the ionization yield to different ionic states in a polyatomic molecule. The results are interpreted in terms of a competition between two types of nonadiabatic dynamics: multiphoton resonance and internal conversion.

Keywords: ultrafast laser; strong field; resonance internal; internal conversion

Journal Title: Physical Review A
Year Published: 2021

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