The authors show theoretically and experimentally how the time-varying phase or frequency of a chirped strong-field ultrafast laser pulse can be used to control the ionization yield to different ionic… Click to show full abstract
The authors show theoretically and experimentally how the time-varying phase or frequency of a chirped strong-field ultrafast laser pulse can be used to control the ionization yield to different ionic states in a polyatomic molecule. The results are interpreted in terms of a competition between two types of nonadiabatic dynamics: multiphoton resonance and internal conversion.
               
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