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Time-dependent Hartree-Fock study of electron-hole interaction effects on high-order harmonic generation from periodic crystals

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We investigate the multielectron effects on high-harmonic generation from solid-state materials using the time-dependent Hartree-Fock theory. We find qualitative change in harmonic spectra, in particular, multiple-plateau formation at significantly lower… Click to show full abstract

We investigate the multielectron effects on high-harmonic generation from solid-state materials using the time-dependent Hartree-Fock theory. We find qualitative change in harmonic spectra, in particular, multiple-plateau formation at significantly lower laser intensities than within the independent-electron approximation. We reveal its origin in terms of interband polarization, i.e, electron-hole polarization, enabling interband excitation at remote crystal momenta via Coulomb potential.

Keywords: dependent hartree; effects high; harmonic generation; time dependent; electron hole; hartree fock

Journal Title: Physical Review A
Year Published: 2017

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