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Ultrahigh-Resolution Direct-Frequency-Comb Spectrometer

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High-resolution broadband spectroscopy is crucial for studying complex molecular structures and accurately retrieving the line shapes associated with their energy levels. These line shapes carry vital information about a molecule's… Click to show full abstract

High-resolution broadband spectroscopy is crucial for studying complex molecular structures and accurately retrieving the line shapes associated with their energy levels. These line shapes carry vital information about a molecule's thermodynamic properties such as temperature, pressure, and concentration, which are desirable for $e.g.$ the petroleum industry, environmental monitoring, and medical breath analysis. This study shows how to obtain a molecular spectrum with about 80 kHz of resolution and 7.86 MHz of spectral sampling. The promising high-resolution technique allows complete gas characterization by simultaneously measuring thermodynamic properties and analyzing composition.

Keywords: direct frequency; resolution; comb spectrometer; resolution direct; ultrahigh resolution; frequency comb

Journal Title: Physical review applied
Year Published: 2020

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