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Interseries transitions between Rydberg excitons in Cu2O

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We investigate the infrared optical transitions between excitons of the yellow, green and blue series in the cuprous oxide Cu$_{\mathrm{2}}$O. We show that in many cases the dipole approximation is… Click to show full abstract

We investigate the infrared optical transitions between excitons of the yellow, green and blue series in the cuprous oxide Cu$_{\mathrm{2}}$O. We show that in many cases the dipole approximation is inadequate and, in particular, that it breaks down in yellow-blue transitions even for moderate principal quantum numbers of $n \approx 10$. The interband matrix elements of the transition operator needed for the evaluation of the excitonic transition strengths are derived from known as well as from fitted band parameters.

Keywords: rydberg excitons; excitons cu2o; transitions rydberg; interseries transitions

Journal Title: Physical Review B
Year Published: 2019

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