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Exciton transport enhancement across quantum Su-Schrieffer-Heeger lattices with quartic nonlinearity

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In the present work we discuss the propagation of excitons across a one-dimensional Su-Schrieffer-Heeger lattice, which possesses both harmonic oscillations and weak quartic anharmonicities. When quantizing these vibrational degrees of… Click to show full abstract

In the present work we discuss the propagation of excitons across a one-dimensional Su-Schrieffer-Heeger lattice, which possesses both harmonic oscillations and weak quartic anharmonicities. When quantizing these vibrational degrees of freedom we identify several phonon-conserving nonlinearities, each one with a different impact on the excitonic transport. Our analysis identifies a dominant nonlinear correction to the phonon hopping which leads to a strong enhancement of exciton conduction compared to a purely linear vibrational dynamics. Thus quartic lattice nonlinearities can be exploited to induce transitions from localized to delocalized transport, even for very weak amplitudes.

Keywords: transport; schrieffer heeger; exciton transport

Journal Title: Physical Review B
Year Published: 2019

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