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Time-resolved resonant inelastic x-ray scattering in a pumped Mott insulator

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Collective excitations contain rich information about photoinduced transient states in correlated systems. In a Mott insulator, charge degrees of freedom are frozen but can be activated by photodoping. The energy-momentum… Click to show full abstract

Collective excitations contain rich information about photoinduced transient states in correlated systems. In a Mott insulator, charge degrees of freedom are frozen but can be activated by photodoping. The energy-momentum distribution of the charge excitation spectrum reflects the propagation of charge degrees of freedom, and provides information about the interplay among various intertwined instabilities at the time scale set by the pump. To reveal the charge excitations out of equilibrium, we simulate the time-resolved x-ray absorption and resonant inelastic x-ray scattering using a Hubbard model. After pump, the former resolves photodoping, while the latter provides finite-momentum collective excitations. With the information about the intermediate state, trRIXS deciphers these excitations from different origins, including the bimagnon, Mott-gap excitations, doublon and single-electron in-gap states, and anti-Stokes relaxations during an ultrafast pump. This work provides a theoretical foundation for existing and future trRIXS experiments.

Keywords: mott insulator; time resolved; time; ray scattering; inelastic ray; resonant inelastic

Journal Title: Physical Review B
Year Published: 2020

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