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Critical temperature and low-energy excitations in gapped spin systems with defects

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We discuss theoretically the magnetically ordered phase induced by magnetic and nonmagnetic impurities in three-dimensional and quasi-low-dimensional systems with singlet ground states separated by a gap from excited triplet states.… Click to show full abstract

We discuss theoretically the magnetically ordered phase induced by magnetic and nonmagnetic impurities in three-dimensional and quasi-low-dimensional systems with singlet ground states separated by a gap from excited triplet states. Using ideas of the percolation theory, we estimate the transition temperature ${T}_{N}(n)$ to the N\'eel phase at a small concentration $n$ of defects, derive the density of states of low-energy elementary excitations, and examine the contribution of these excitations to the specific heat and magnetization. Our expressions for ${T}_{N}(n)$ and for the specific heat describe well available experimental findings obtained in various appropriate systems: spin-$\frac{1}{2}$ dimer materials, spin-ladder compounds, spin-Peierls, and Haldane chain materials. However, our expression for ${T}_{N}(n)$ differs considerably from many of those proposed before.

Keywords: temperature low; low energy; critical temperature; energy excitations; temperature

Journal Title: Physical Review B
Year Published: 2021

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