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Graphene valley polarization as a function of carrier-envelope phase in few-cycle laser pulses and its footprints in harmonic signals

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We consider coherent dynamics of graphene charged carriers exposed to an intense few-cycle linearly polarized laser pulse. The results, obtained by solving the generalized semiconductor Bloch equations numerically in the… Click to show full abstract

We consider coherent dynamics of graphene charged carriers exposed to an intense few-cycle linearly polarized laser pulse. The results, obtained by solving the generalized semiconductor Bloch equations numerically in the Hartree-Fock approximation, taking into account many-body Coulomb interaction, demonstrate strong dependence of the valley polarization on the carrier-envelope phase (CEP), which is interpolated by the simple sinusoidal law. Then we consider harmonic generation in multi-cycle laser field by graphene preliminary exposed to an intense few-cycle laser pulse. We show that the second harmonic's intensity is a robust observable quantity that provides a gauge of CEP for pulse durations up to two optical cycles, corresponding to 40 $\mathrm{fs}$ at the wavelength of 6.2 $\mathrm{\mu m}$.

Keywords: envelope phase; cycle; laser; valley polarization; cycle laser; carrier envelope

Journal Title: Physical Review B
Year Published: 2023

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